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E-mail: catherine. The recent advent of CLRP techniques such as nitroxide-mediated polymerization NMP , 4 atom-transfer radical polymerization ATRP 5,6 and reversible-addition fragmentation chain transfer RAFT , 7 which are compatible with a large range of functional monomers, has opened new prospects in the polysaccharide-based material area. By controlling the grafting density, the length and the composition of the grafted chains, new hybrid materials with finely tuned properties are now available that enlarge the range of sustainable materials. To our knowledge, only Daly et al. Nevertheless, NMP is nowadays maybe one of the most convenient CLRP techniques since it is a monocomponent initiating system that does not require any catalyst. This method allows elaboration of complex architectures such as block or star copolymers as well as chitosan-based grafted copolymers.

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